세미나 Seminars

2018.09.07 18:05

9월13일(목) 대학원세미나 Prof. Y. Nakao(Department of Material Chemistry, Graduate School of Engineering, Kyoto University)

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초청강사 Prof. Y. Nakao
소속 Department of Material Chemistry, Graduate School of Engineering, Kyoto University
일시 2018년 9월 13일(목) 오후 5시
장소 아산이학관 331호

Cooperative Metal Catalysis for Efficient Organic Synthesis

 

A number of useful CC and Cheteroatom bond forming reactions have been developed by taking advantages of varied reaction modes of metal complexes. We have envisaged that the power of metal catalysis can be brought out further by designing cooperative catalysis derived from two or more different metal complexes. We show that some novel CC and Cheteroatom bond forming reactions are enabled by doubly activating cooperative catalysis with late transition metals and Lewis acids. Examples include cyanofunctionalization,13 hydro(hetero)arylation,4 hydrocarbamoylation,5 and borylation6 reactions through CCN, OCN, NCN, and CH functionalization by nickel, palladium, or iridium/Lewis acid cooperative double activation catalysis.



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1.  Y. Nakao, Bull. Chem. Soc. Jpn. 2012, 85, 731. 2 D. C.Koester, M. Kobayashi, D. B. Werz, Y. Nakao, J. Am. Chem. Soc. 2012, 134, 6544. 3 Y. Miyazaki, N. Ohta, K. Semba, Y. Nakao, J. Am. Chem. Soc. 2014, 136, 3732. 4 S. Okumura, S. Tang, T. Saito, K. Semba, S. Sakaki, Y. Nakao, J. Am. Chem. Soc. 2016, 138, 14699. 5 Y. Miyazaki, Y. Yamada, Y. Nakao, T. Hiyama, Chem. Lett. 2012, 41, 298. 6 L. Yang, K. Semba, Y. Nakao, Angew. Chem. Int. Ed. 2017, 56, 4853.

 


20180913_대학원세미나_Prof. Y. Nakao.pdf


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